Header menu link for other important links
X
Infrequent occurrence of new particle formation at a semi-rural location, Gadanki, in tropical Southern India
, Raghunathan Ravikrishna,
Published in Elsevier Ltd
2014
Volume: 94
   
Pages: 264 - 273
Abstract
We report first measurements of ultrafine particles from a semi-rural location, Gadanki, from tropical Southern India. Measurements of particle number size distributions in the diameter range of 5nm-32μm were performed during 2 May-31 July 2012. The mean number concentrations of nucleation (NNUC), Aitken (NAIT), accumulation (NACCU), and total particles (NTOT) at this site were (1.1±0.9)×103cm-3, (2.2±1.3)×103cm-3, (1.5±1.2)×103cm-3 and (4.8±2.4)×103cm-3, respectively, comparable to other rural to semi-rural locations globally and declined as the season progressed, perhaps due to wet removal of aerosols with onset of monsoon in early June. Particle bursts in the nucleation mode size range (5-25nm), followed by a sustained growth in size were observed very rarely (only 5 out of 79 observation days) at this site, less frequently than at most other locations around the world during May-July. Most factors affecting new particle formation (NPF) were similar on NPF and nonNPF event days, such as condensation sink, relative humidity, temperature, wind speed and direction, and mixing layer height. Thus, the infrequent occurrence of NPF at our site appeared to be linked to lower precursor gas concentrations and weak gas-phase oxidation chemistry due to diminished solar radiation on persistently cloudy days with the onset of the monsoon in early June over this region. The derived particle growth rates (GR>5nm) and formation rates of 5nm particles (J5) ranged from 2.2 to 4.7nmh-1 and 0.4-2.4cm-3s-1, with a mean and standard deviation of 3.4±0.9nmh-1 and 1.2±2.3cm-3s-1, respectively, comparable to previous investigations at rural to semi-rural locations. The observed behavior in aerosol and meteorological parameters on NPF and nonNPF event days appeared to be distinctive compared to other rural to urban locations across the globe. However, this distinct behavior is limited and restricted to this site and season of the year, and should therefore not be generalized over a larger spatio-temporal scale. This emphasizes the need for long-term aerosol and precursor measurements over this and other regions of India. © 2014 Elsevier Ltd.
About the journal
JournalData powered by TypesetAtmospheric Environment
PublisherData powered by TypesetElsevier Ltd
ISSN13522310
Open AccessNo
Concepts (40)
  •  related image
    Aerosols
  •  related image
    Atmospheric thermodynamics
  •  related image
    Nucleation
  •  related image
    Particle size analysis
  •  related image
    Sun
  •  related image
    MEAN AND STANDARD DEVIATIONS
  •  related image
    Meteorological parameters
  •  related image
    NEW PARTICLE FORMATION
  •  related image
    PARTICLE GROWTH RATES
  •  related image
    PARTICLE NUMBER SIZE DISTRIBUTION
  •  related image
    SEMI-RURAL
  •  related image
    SPATIO-TEMPORAL SCALE
  •  related image
    WIND SPEED AND DIRECTIONS
  •  related image
    Tropics
  •  related image
    Aerosol formation
  •  related image
    Aerosol property
  •  related image
    Concentration (composition)
  •  related image
    Particle size
  •  related image
    RURAL ATMOSPHERE
  •  related image
    Seasonality
  •  related image
    Size distribution
  •  related image
    Solar radiation
  •  related image
    Aerosol
  •  related image
    Article
  •  related image
    Gas
  •  related image
    Height
  •  related image
    Humidity
  •  related image
    India
  •  related image
    Meteorology
  •  related image
    NEW PARTICLE FORMATION
  •  related image
    Oxidation
  •  related image
    Precursor
  •  related image
    Priority journal
  •  related image
    Rural area
  •  related image
    Season
  •  related image
    Temperature
  •  related image
    Velocity
  •  related image
    Wind
  •  related image
    GADANKI
  •  related image
    Tamil nadu