Tribological behaviors of plasma-sprayed conventional and nanostructured Cr₂O₃–3%TiO₂ ceramic coatings (i.e., CC3T and NC3T, respectively) using pin on disc type dry sliding and pot type slurry erosion test were investigated in the present work. The experimental results indicated that there were two main wear mechanisms, plastic smearing and adhesive tearing, in the worn coatings under dry sliding. Plastic smearing corresponded to a lower average friction coefficient and wear rate, while adhesive tearing corresponded to higher values. The erosive environment selected for the slurry erosion experiments include 10, 20 and 30% of SiO₂ slurry concentrations in water with particle size 75–106 μm. The main damage mechanism observed in all the coatings submitted to slurry erosion were the formation and propagation of brittle cracks resulting in the detachment of coating surface material. Microstructural investigation was also carried to investigate the wear and erosion mechanism of the coatings using FE-SEM and EDS analysis. Properties like microhardness and porosity were also investigated for these coatings. Tribological performance of NC3T was better as compared to CC3T as observed in the present work.