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Nonlinear behavior of coupled reactor-separator systems with azeotropic vapor-liquid equilibriums (VLEs): Comparison of different control strategies
Published in
2006
Volume: 45
   
Issue: 3
Pages: 1019 - 1028
Abstract
In this paper, we discuss the behavior of a coupled reactor - separator system. The reactor is modeled as a continuously stirred tank reactor (CSTR) sustaining an elementary first-order reaction and the separator as a single-stage flash unit. The coupling occurs via the recycling of the bottoms stream from the downstream separator to the upstream reactor. The emphasis in this paper is on studying the behavior of the coupled system when the vapor - liquid equilibrium (VLB) of the mixture has an azeotrope. Consequently, the bottoms stream can be reactant-rich or reactant-lean. Different control strategies for the operation of the reactor and separator are discussed. The stability of the steady states is analyzed analytically for each strategy. Physical explanations for the stabilty results are presented. Generally, the recycle of the reactant lean stream is observed to cause instability. © 2006 American Chemical Society.
About the journal
JournalIndustrial and Engineering Chemistry Research
ISSN08885885
Open AccessNo
Concepts (12)
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    AZEOTROPES
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    Nonlinear systems
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    Reaction kinetics
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    Recycling
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    Separators
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    Tanks (containers)
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    CONTINUOUSLY STIRRED TANK REACTORS (CSTR)
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    FIRST-ORDER REACTION
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    LEAN STREAM
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    SINGLE-STAGE FLASH UNIT
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    Chemical reactors
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    AZEOTROPES