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Studies on the reactivity of new types of tetracyclic-1, 5-benzoxazepines: Part V
Sukuru Raghu Ramadas
Published in
2001
Volume: 38
   
Issue: 2
Pages: 383 - 386
Abstract
The syntheses of tetracyclic 1, 5-benzoxazepines 3a-e from heterocyclic β-chloroaldehydes 1a-e and 2-aminophenol are reported herein (Scheme I). Attempted lithium aluminium hydride (LiAlH4) reduction of the imine double bond in 3a-e failed to furnish the corresponding saturated compounds 5a-e. Attempted catalytic hydrogenation of 3a-e in the presence of acetic acid and acetic anhydride gave surprisingly only the acetoxy derivatives 6a-e in high yields (Scheme II). Base catalysed hydrolysis of acetoxy derivatives 6a-e furnished, as expected, the corresponding phenolic derivatives 7a-e, in moderate yields. Attempted cyclofunctionalization of 3a-e either with mercaptoacetic acid or its methyl ester to obtain the new pentacyclic heterocycles 4a-e was, however, not successful.
About the journal
JournalJournal of Heterocyclic Chemistry
ISSN0022152X
Open AccessNo
Concepts (18)
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    2 AMINOPHENOL
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    3 METHOXYBENZOFURO[3,2 B]BENZOXAZEPINE
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    6,7 DIHYDRO[1]BENZOTHIEPINO[5,4 B][1,5]BENZOXAZEPINE
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    6,7 DIHYDRO[1]BENZOXEPINO[5,4 B][1,5]BENZOXAZEPINE
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    6H [1]BENZOPYRANO[4,3 B][1,5]BENZOXAZEPINE
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    6H [1]BENZOTHIOPYRANO[4,3 B][1,5]BENZOXAZEPINE
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    Acetic acid
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    ACETIC ANHYDRIDE
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    Aldehyde derivative
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    Heterocyclic compound
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    Lithium derivative
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    TETRACYCLIC 1,5 BENZOXAZEPINE DERIVATIVE
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    Unclassified drug
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    Article
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    DRUG HYDROLYSIS
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    Drug structure
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    Drug synthesis
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    Hydrogenation