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Observation of spin glass state in weakly ferromagnetic Sr 2FeCoO 6 double perovskite
Published in
2012
Volume: 111
   
Issue: 5
Abstract
A spin glass state is observed in the double perovskite oxide Sr 2FeCoO 6 prepared through sol-gel technique. Initial structural studies using x rays reveal that the compound crystallizes in tetragonal I4/m structure with lattice parameters, a 5.4609(2) Å and c 7.7113(7) Å. The temperature dependent powder x ray diffraction data reveal no structural phase transition in the temperature range 10-300 K. However, the unit cell volume shows an anomaly coinciding with the magnetic transition temperature thereby suggesting a close connection between lattice and magnetism. Neutron diffraction studies and subsequent bond valence sums analysis show that in Sr 2FeCoO 6, the B site is randomly occupied by Fe and Co in the mixed valence states of Fe 3+/Fe 4+ and Co 3+/Co 4+. The random occupancy and mixed valence sets the stage for inhomogeneous magnetic exchange interactions and in turn, for the spin glass state in this double perovskite, which is observed as an irreversibility in temperature dependent dc magnetization at T f ∼ 75 K. Dynamical scaling analysis of ′(T) yields a critical temperature T ct 75.14(8) K and an exponent z 6.2(2) typical for spin glasses. The signature of presence of mixed magnetic interactions is obtained from the thermal hysteresis in magnetization of Sr 2FeCoO 6. Combining the neutron and magnetization results of Sr 2FeCoO 6, we deduce that Fe is in low spin state while Co is in both low spin and intermediate spin states. © 2012 American Institute of Physics.
About the journal
JournalJournal of Applied Physics
ISSN00218979
Open AccessNo
Authors (4)
Concepts (28)
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    BOND VALENCE SUMS
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    Critical temperatures
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    Dc magnetization
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    DOUBLE PEROVSKITE OXIDE
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    Double perovskites
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    DYNAMICAL SCALING
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    INTERMEDIATE SPINS
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    Magnetic exchange interactions
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    Magnetic interactions
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    Magnetic transition temperature
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    Mixed valence
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    Mixed valence state
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    Powder x ray diffraction
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    SOL-GEL TECHNIQUE
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    Spin glass state
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    Spin state
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    Structural phase transition
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    Structural studies
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    Temperature dependent
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    Temperature range
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    Thermal hysteresis
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    UNIT-CELL VOLUME
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    Magnetization
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    Perovskite
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    Sol-gels
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    Spin dynamics
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    X ray diffraction
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    Spin glass