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A facile room-temperature synthesis of gold nanowires by oxalate reduction method
S. Navaladian, C. M. Janet, Balasubramanian Viswanathan, Thirukkallam Kanthadai Varadarajan, Ram Prasad Viswanath
Published in
2007
Volume: 111
   
Issue: 38
Pages: 14150 - 14156
Abstract
Polycrystalline gold nanowires were synthesized by a simple chemical reduction method using potassium oxalate as the reducing and capping agent along with polyvinylpyrrolidone (PVP) as the co-capping agent at room temperature. Different molar concentration ratios of HAuCl4 and potassium oxalate were studied for the synthesis of Au nanowires. Kinetics studies for Au colloid formation were carried out using UV-vis spectroscopic technique for the various concentration ratios of the reactants. As the concentration of oxalate was increased, the rate of reduction as well as particle growth was found to increase. XRD and TEM analyses revealed the formation of polycrystalline Au nanowires with a preferential growth of the {111} facet. In the absence of PVP, no Au colloid was formed. Studies revealed that the formation of the Au nanowire was due to the bridging nature of the oxalate dianion. The formation of Pt nanowires further supported the role of oxalate when the same method was adopted for the synthesis of Pt nanowires without using PVP. A plausible mechanism was proposed for the formation of Au nanowires explaining the role of oxalate. © 2007 American Chemical Society.
About the journal
JournalJournal of Physical Chemistry C
ISSN19327447
Open AccessNo
Concepts (12)
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    Colloids
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    Gold
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    Polycrystalline materials
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    Potassium compounds
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    Reduction
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    Spectroscopy
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    Synthesis (chemical)
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    Capping agent
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    CHEMICAL REDUCTION METHOD
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    MOLAR CONCENTRATION RATIOS
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    OXALATE REDUCTION METHOD
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    Nanowires